Pt decorated amorphous RuIr alloys as high efficiency electrocatalyst for methanol oxidation

Loading...
Thumbnail Image

Date

2012

Journal Title

Journal ISSN

Volume Title

Publisher

The Electrochemical Society

Abstract

This study focuses primarily on improving the utilization and activity of anodic catalysts for methanol electro-oxidation. The Direct Methanol Fuel Cell (DMFC) anodic catalyst, a carbon supported Pt decorated amorphous RuIr nanoparticles catalyst (Pt@RuIr/C) was prepared by a two-step reduction method. The structure of Pt@RuIr/C nanoparticles was confirmed by Transmission Electron Microscopy (TEM) and X-ray Diffraction (XRD). The Pt@RuIr electrocatalysts exhibited good uniformity in distribution. Cyclic Voltammetry experiments showed that under the same quality of noble-metal, the Pt@RuIr/C catalyst had higher activity than the PtRuIr/C catalyst for methanol oxidation. It was also shown that the as-prepared structure of the Pt decorated amorphous RuIr alloys could obviously decrease the usage of noble-metal and enhance its catalytic activity at the same time.

Description

Keywords

Anodic catalyst, Methanol electro-oxidation, Reduction method, Transmission Electron Microscopy (TEM), X-ray Diffraction (XRD)

Citation

Ma, Y.J. et al. (2012). Pt decorated amorphous RuIr alloys as high efficiency electrocatalyst for methanol oxidation. ECS Transactions, 50(2): 1943 – 1950